The key to understanding tongues is through understanding the dividing of spirit, soul and body.

To speak the tongue of angels is the tongue of spirit, from your inner women or inner man which is your spirit like the angels who are spirits. To do this God gives revelation to do it in your spirit intuitively (not by gibberish babble), and this language of the spirit is transmitted to the soul through gifting of other languages to speak words of God to share the Word to those of other languages.

This is very precise.